They contain a compound called capsaicin (or related compounds) which is produced probably as a deterrent to herbivores (shame then that we as a human race have acquired a taste for these things, isn’t it?). The painful sensation linked to the consumption of capsaicin is due to its activation of neurons through a receptor (the vanilloid receoptor).
Does this answer your question? Do you like your curries hot or do you prefer milder ones?
I don’t know if you know but there is actually a scale which chilli heat is measured on. It’s called the Scoville scale and measures the amount of capsaicin (that compound Blank was talking about) in the chilli.
Blanka and Emma covered this perfectly, so here’s my only bonus fact: capsaicin is used in pepper sprays, which the police sometimes use (and people use themselves in the US and other countries to protect themselves). Pepper spray is pretty dangerous stuff, partly because capsaicin is so powerful!
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